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Published 08:00 14 May 2020 BST
Updated 08:07 14 May 2020 BST
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The former child star has also requested that the pre-nuptial agreement she and Olivier signed prior to marrying be enacted, TMZ said.
Mary-Kate and Olivier, whose half-brother is former French president Nicolas Sarkozy, first began dating in 2012 and married in New York in November 2015.
Having first risen to fame at the age of one, Mary-Kate and twin sister Ashley announced their retirement from acting in 2012.
They now run luxury fashion brands The Row and Elizabeth and James.Celebrity